Reaction fronts of the autocatalytic hydrogenase reaction
We have built a model to describe the hydrogenase catalyzed, autocatalytic, reversible hydrogen oxidation reaction where one of the enzyme forms is the autocatalyst. The model not only reproduces the experimentally observed front properties, but also explains the found hydrogen ion dependence. Furth...
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Main Authors: | |
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Format: | Article |
Published: |
2018
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Series: | JOURNAL OF CHEMICAL PHYSICS
148 No. 16 |
doi: | 10.1063/1.5022359 |
mtmt: | 3372671 |
Online Access: | http://publicatio.bibl.u-szeged.hu/15381 |
Summary: | We have built a model to describe the hydrogenase catalyzed, autocatalytic, reversible hydrogen oxidation reaction where one of the enzyme forms is the autocatalyst. The model not only reproduces the experimentally observed front properties, but also explains the found hydrogen ion dependence. Furthermore, by linear stability analysis, two different front types are found in good agreement with the experiments. Published by AIP Publishing. |
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Physical Description: | Paper 165103-8 p |
ISSN: | 0021-9606 |